Calibration-free wavelength modulation spectroscopy based on even-order harmonics

Multiplexed absorption tomography with calibration-free wavelength modulation spectroscopy

Odd harmonics with wavelength modulation spectroscopy for recovering gas absorbance shape.

In this paper, a new method for recovering gas absorbance shape using wavelength modulation spectroscopy is proposed. We have mathematically proven that the gas absorbance shape can be directly recovered using the data of X and Y components of odd harmonics, regardless of the value of the modulation depth. The transitions of NH(3) near 1531 nm are selected to recover the absorbance shape using ...

Ramsey-type spectroscopy with high-order harmonics.

We present an experiment where Ramsey-type spectroscopy is applied to autoionizing states of krypton by using the ninth harmonic (88 nm) of a femtosecond Ti:sapphire laser. The ionization process, detected by an electron-energy spectrometer, shows the characteristic quantum interference pattern. The behavior of the fringe contrast compares favorably with a simple essential-state model, whose pa...

In Situ H2o and Temperature Detection Close to Burning Biomass Pellets Using Calibration-free Wavelength Modulation Spectroscopy

The design and application of an H2O/temperature sensor based on scanned calibration-free wavelength modulation spectroscopy (CF-WMS) and a single tunable diode laser at 1.4 μm is presented. The sensor probes two H2O absorption peaks in a single scan and simultaneously retrieves H2O concentration and temperature by least-squares fitting simulated 1f-normalized 2f-WMS spectra to measured 2f/1f-W...

Quasi-phase-matching of only even-order high harmonics.

High harmonic spectrum of a quasi-monochromatic pump that interacts with isotropic media consists of only odd-order harmonics. Addition of a secondary pump, e.g. a static field or the second harmonic of the primary pump, can results with generation of both odd and even harmonics of the primary pump. We propose a method for quasi-phase matching of only the even-order harmonics of the primary pum...